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MATERIALS SCIENCE AND TECHNOLOGY. SEMICONDUCTORS
Название Thermoelectric Properties of Spark Plasma Sintering Synthesized (Bi,Sb)2Te3 Based Bulk Thermoelectric Material
Автор I. A. Drabkin, V. V. Karataev, V. B. Osvensky, Yu. N. Parkhomenko, A. I. Sorokin, L. P. Bulat, G. I. Pivovarov, V. T. Bublik, N. Yu. Tabachkova
Информация об авторе

Giredmet

I. A. Drabkin

V. V. Karataev

V. B. Osvensky
Yu. N. Parkhomenko

A. I. Sorokin

L. P. Bulat

 

Technical Institute for Ultrahard and New Carbon Materials
G. I. Pivovarov

 

National University of Science and Technology MISiS

V. T. Bublik

N. Yu. Tabachkova

Реферат

Thermoelectric properties of (Bi,Sb)2Te3 nanostructured bulk material as a function of composition and spark plasma sintering temperature were investigated. The Bi0,4Sb1,6Te3 alloys at sintering temperature 450—500 °C with ZT=1,25—1,28 figure of merit was fabricated. Thermoelectric properties ad a function of sintering temperature above 400 °C correlate with fine structure change. It was found that point structure defects introduce essential contribution to the formation of nanostructured material thermoelectric properties.

Ключевые слова Spark plasma sintering, nanostructured material, bismuth telluride, thermoelectric properties, structural defects, Harman method
Библиографический список

1. Poudel, B. High−thermoelectric performance of nanostructured bismuth antimony telluride bulk alloys / B. Poudel, Q. Hao, Y. Ma, X. Y. Lan, A. Minnich, B. Yu, X. Yan, D. Z. Wang, A. Muto, D. Vashaee, X. Y. Chen, J. M. Liu, M. S. Dresselhaus, G. Chen, Z. F. Ren // Science. − 2008. − V. 320, N 5876. − P. 634—638.
2. Fan, S. J. R−type Bi0,4Sb1,6Te3 nanocomposites with enhanced figure of merit / S. J. Fan, J. Zhao, J. Guo, Q. Yan, J. Ma, H. Hong // Appl. Phys. − 2010. − V. 96, N 182104. − P. 456—459.
3. Bublik, V. T. Struktura ob"emnogo termoelektricheskogo materiala na osnove (Bi,Sb)2Te3, poluchennaya metodom iskrovogo plazmennogo spekaniya / V. T. Bublik, I. A. Drabkin, V. V. Karataev, M. G. Lavrent'ev, V. B. Osvenskiy, Yu. N. Parkhomenko, G. I. Pivovarov, A. I. Sorokin, N. Yu. Tabachkova // Izv. vuzov. Materialy elektron. tekhniki. − 2012. − № 3. − S. 10—17.
4. Abryutin, V. N. Izmerenie termoelektricheskikh obraztsov metodom Kharmana / V. N. Abryutin, I. A. Drabkin, I. I. Maronchuk, V. B. Osvenskiy // IX Mezhgosudarstv. seminar «Termoelektriki i ikh primeneniya». − SPb: FTI im. A.F. Ioffe RAN, 2004. − S. 303—308.
5. Keawprak, N. Effect of sintering temperature on the thermoelectric properties of pulse discharge sintered (Bi0,24Sb0,76)2Te3 alloy / N. Keawprak, Z. M. Suna, H. Hashimoto, M. W. Barsoumb // J. Alloys and Compounds. − 2005. −V. 397, N 2. − R. 236—244.
6. Bulat, L. P. Vliyanie rasseyaniya na granitsakh na teploprovodnost' nanostrukturirovannogo poluprovodnikovogo materiala na osnove tverdogo rastvora BixSb2−xTe3 / L. P. Bulat, I. I. Drabkin, V. V. Karataev, V. B. Osvenskiy, D. A. Pshenay−Severin // FTT. − 2010. − T. 52, № 9. − S. 1712—1716.
7. Zhao, D. Enhanced thermoelectric and mechanical properties in textured n−type Bi2Te3 prepared by spark plasma sintering / D. Zhao, B. P. Zhang, J. F. Li, H. L. Zhang, W. S. Liu // Solid State Sciences. − 2008. − N 10. − R. 651—658.
8. Lan, Y. Structure study of bulk nanograined thermoelectric bismuth antimony telluride / Y. Lan, B. Poudel, Y. Ma, M. S. Dresselhaus, G. Chen, Z. Ren // Nano Lett. − 2009. − V. 9, N 4. − P. 1419—1422.
9. Bublik, V. T. Transportnye svoystva v oblasti temperatur 10—300 K nanostrukturirovannogo p−Bi0,5Sb1,5Te3, poluchennogo metodom iskrovogo plazmennogo spekaniya / V. T. Bublik, Z. M. Dashevskiy, I. A. Drabkin, V. V Karataev, V. B. Osvenskiy, G. I. Pivovarov, D. A. Pshenay−Severin, N. Yu. Tabachkova // XII Mezhgosudarstv. seminar «Termoelektriki i ikh primeneniya». − SPb: FTI im. A. F. Ioffe RAN, 2010. − S. 250—252.

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